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71.
We consider the MAP/PH/N retrial queue with a finite number of sources operating in a finite state Markovian random environment. Two different types of multi-dimensional Markov chains are investigated describing the behavior of the system based on state space arrangements. The special features of the two formulations are discussed. The algorithms for calculating the stationary state probabilities are elaborated, based on which the main performance measures are obtained, and numerical examples are presented as well. 相似文献
72.
Ling Wang Xiao-Tong Wang Jia-Huan Zhong Dr. Kang Xiao Dr. Ting Ouyang Prof. Zhao-Qing Liu 《Chemistry (Weinheim an der Bergstrasse, Germany)》2021,27(18):5796-5802
The high charge–discharge voltage gap is one of the main bottlenecks of zinc–air batteries (ZABs) because of the kinetically sluggish oxygen reduction/evolution reactions (ORR/OER) on the oxygen electrode side. Thus, an efficient bifunctional catalyst for ORR and OER is highly desired. Herein, honeycomb-like MnCo2O4.5 spheres were used as an efficient bifunctional electrocatalyst. It was demonstrated that both ORR and OER catalytic activity are promoted by MnIV-induced oxygen vacancy defects and multiple active sites. Importantly, the multivalent ions present in the material and its defect structure endow stable pseudocapacitance within the inactive region of ORR and OER; as a result, a low charge–discharge voltage gap (0.43 V at 10 mA cm−2) was achieved when it was employed in a flexible hybrid Zn-based battery. This mechanism provides unprecedented and valuable insights for the development of next-generation metal–air batteries. 相似文献
73.
Hui Shi Ziheng Wang Dr. Qin Ouyang Prof. Jianwei Hao Dr. Xianbo Huang 《Chemistry (Weinheim an der Bergstrasse, Germany)》2021,27(30):8030-8039
Retaining nitrogen for polyacrylonitrile (PAN) based carbon anode is a cost-effective way to make full use of the advantages of PAN for sodium-ion batteries (SIBs). Here, a simple strategy has been successfully adopted to retain N atoms in situ and increase production yield of a novel composite PAZ by mixing 3 wt % of zinc borate (ZB) with poly (acrylonitrile-co-itaconic acid) (PANIA). Among the prepared carbonised fibre (CF) samples, PAZ-CF-700 maintains the highest N content, retaining 90 % of the original N from PANIA. It represents the highest capacity storage contribution (80.55 %) and the lowest impedance Rct (117 Ω). Consequently, the specific capacity increases from 60 mAh g−1 of PANIA-CF-700 to 190 mAh g−1 of PAZ-CF-700 at a current density of 100 mA g−1. At the same time, PAZ-CF-700 exhibits a good rate performance and excellent long-term cycling stability with a specific capacity of 94 mAh g−1 after 4000 cycles at 1.6 A g−1. 相似文献
74.
Recently, a polynomial-based (k, n) steganography and authenticated image sharing (SAIS) scheme was proposed to share a secret image into n stego-images. At the same time, one can reconstruct a secret image with any k or more than k stego-images, but one cannot obtain any information about the secret from fewer than k stego-images. The beauty of a (k, n)-SAIS scheme is that it provides the threshold property (i.e., k is the threshold value), the steganography (i.e., stego-images look like cover images), and authentication (i.e., detection of manipulated stego-images). All existing SAIS schemes require parity bits for authentication. In this paper, we present a novel approach without needing parity bits. In addition, our (k, n)-SAIS scheme provides better visual quality and has higher detection ratio with respect to all previous (k, n)-SAIS schemes. 相似文献
75.
Dr. Ting Ouyang Sheng Huang Xiao-Tong Wang Prof. Zhao-Qing Liu 《Chemistry (Weinheim an der Bergstrasse, Germany)》2020,26(62):14024-14035
One of the most effective ways to cope with the problems of global warming and the energy shortage crisis is to develop renewable and clean energy sources. To achieve a carbon-neutral energy cycle, advanced carbon sequestration technologies are urgently needed, but because CO2 is a thermodynamically stable molecule with the highest carbon valence state of +4, this process faces many challenges. In recent years, electrochemical CO2 reduction has become a promising approach to fix and convert CO2 into high-value-added fuels and chemical feedstock. However, the large-scale commercial use of electrochemical CO2 reduction systems is hindered by poor electrocatalyst activity, large overpotential, low energy conversion efficiency, and product selectivity in reducing CO2. Therefore, there is an urgent need to rationally design highly efficient, stable, and scalable electrocatalysts to alleviate these problems. This minireview also aims to classify heterogeneous nanostructured electrocatalysts for the CO2 reduction reaction (CDRR). 相似文献
76.
We emphasize that it is extremely important for future neutrinoless double-beta(0νββ)decay experiments to reach the sensitivity to the effective neutrino mass|mββ|≈1 meV.With such a sensitivity,it is highly possible to discover the signals of 0νββ decays.If no signal is observed at this sensitivity level,then either neutrinos are Dirac particles or stringent constraints can be placed on their Majorana masses.In this paper,assuming the sensitivity of|mββ|≈1 meV for future 0νββ decay experiments and the precisions on neutrion oscillation parameters after the JUNO experiment,we fully explore the constrained regions of the lightest neutrino mass m1 and two Majorana-type CP-violating phases{ρ,σ}.Several important conclusions in the case of normal neutrino mass ordering can be made.First,the lightest neutrino mass is severely constrained to a narrow range m1∈[0.7,8]meV,which together with the precision measurements of neutrino mass-squared differences from oscillation experiments completely determines the neutrino mass spectrum m2∈[8.6,11.7]meV ing phases is limited to ρ∈[130°,230°],which cannot be obtained from any other realistic experiments.Third,the sum of three neutrino masses is found to beΣ≡m1+m2+m3∈[59.2,72.6]meV,while the effective neutrino mass for beta decays turns out to be mβ≡(|Ue1|2m1^2+|Ue2|2m2^2+|Ue3|2m3^2)1/2∈[8.9,12.6]meV.These observations clearly set up the roadmap for future non-oscillation neutrino experiments aiming to solve the fundamental problems in neutrino physics. 相似文献
77.
A simple,rapid and reliable liquid chromatography–mass spectrometry method for determination of methotrexate in human plasma and its application to therapeutic drug monitoring 下载免费PDF全文
Dan Wu Yixuan Wang Yan Sun Nian Ouyang Jun Qian 《Biomedical chromatography : BMC》2015,29(8):1197-1202
A simple, rapid and reliable liquid chromatography–electrospray ionization tandem mass spectrometry method was established and validated for the determination of methotrexate in human plasma. After a straightforward protein precipitation by acetonitrile–water (70:30, v/v), methotrexate (MTX) and p‐aminoacetophenone (used as internal standard, IS) were separated on a Column C18 column (50 × 2.1 mm, 3 µm; Column Technology, Fremont, CA, USA) using a gradient elution with mobile phase of acetonitrile and 0.03% acetic acid aqueous solution at a flow rate of 0.5 mL/min. The total chromatographic runtime was 5 min for each injection. Quantification detection was performed in a triple‐quadruple tandem mass spectrometer under positive mode monitoring the following mass transitions: m/z 455.3 → 308.3 for MTX and m/z 136.1 → 94.4 for IS. The calibration curve was linear over the range of 0.05–25.0 µmol/L with a lower limit of quantification of 0.05 µmol/L. The intra‐ and interday precisions were <5.2%, the accuracy varied from ?4.1 to 4.5%. The recovery was >94%. The LC‐MS/MS method showed an excellent agreement with the existing HPLC‐UV method using Passing–Bablok regression and Bland–Altman difference plot analysis. The validated LC‐MS/MS can be successfully applied to the routine therapeutic drug monitoring of MTX in clinical laboratories. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
78.
Zhang Menghua Zhang Yongfeng Ouyang Huimin Ma Changhui Cheng Xingong 《Nonlinear dynamics》2020,99(4):2727-2741
Nonlinear Dynamics - An adaptive integral sliding mode control (AISMC) method with payload sway reduction is presented for 4-DOF tower cranes in this paper. The designed controller consists of... 相似文献
79.
80.
The Dieudonn-Manin classification theorem on φ-modules (φ-isocrystals) over a perfect field plays a very important role in p-adic Hodge theory. In this note, in a more general setting we give a new proof of this result, and in the course of the proof, we also give an explicit construction of the Harder-Narasimhan filtration of a φ-module. 相似文献